Original Article
  • Preparation of PVA/Graphene Oxide/Fe3O4 Magnetic Microgels as an Effective Adsorbent for Dye Removal

  • Seongmoon Go*, Keunseong Kim*, Eunsol Wi*, Rae-Su Park***, Hong-Ryun Jung****,
    Changhun Yun*,**†, Mincheol Chang*,**†

  • * Department of Polymer Engineering, Graduate School, Chonnam National University, Gwangju 61186, Korea
    ** School of Polymer Science and Engineering, Chonnam National University, Gwangju 61186, Korea
    *** Department of Chemical Engineering, Chosun University, Gwangju 61452, Korea
    **** Industry-University Cooperation Foundation, Chonnam National University, Gwangju 61186, Korea

  • 폴리바이닐알코올/그래핀 옥사이드/산화철 자성 마이크로겔을 이용한 염료 제거

  • 고성문* · 김근성* · 위은솔*· 박래수***· 정홍련****· 윤창훈*,**† · 장민철*,**†

  • This article is an open access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/by-nc/4.0) which permits unrestricted non-commercial use, distribution, and reproduction in any medium, provided the original work is properly cited.

References
  • 1. Gil, T.H., Lee, W.H., and Ahn, J.-H., “Adsorption of Methylene Blue from Aqueous Solution by Pumpkin-Seed Residue,” Korean Society of Environmental Engineers, Vol. 42, No. 1, 2020, pp.10-18.
  •  
  • 2. Katheresan, V., Kansedo, J., and Lau, S.Y., “Efficiency of Various Recent Wastewater Dye Removal Methods: A Review,” Journal of Environmental Chemical Engineering, Vol. 6, No. 4, 2018, pp. 4676-4697.
  •  
  • 3. Lee, J.J., “Isotherm, Kinetic, Thermodynamic and Competitive for Adsorption of Brilliant Green and Quinoline Yellow Dyes by Activated Carbon,” Korean Chemical Engineering Research, Vol. 59, No. 4, 2021, pp. 565-573.
  •  
  • 4. Hussain, S., Kamran, M., Khan, S.A., Shaheen, K., Shah, Z., Suo, H., Khan, Q., Shah, A.B., Rehman, W.U., Al-Ghamdi, Y.O., and Ghani, U., “Adsorption, Kinetics and Thermodynamics Studies of Methyl Orange Dye Sequestration Through Chitosan Composites Films”, International Journal of Biological Macromolecules, Vol. 168, 2021, pp. 383-394.
  •  
  • 5. Cheng, Z., Liao, J., He, B., Zhang, F., Zhang, F., Huang, X., and Zhou, L., “One-step Fabrication of Graphene Oxide Enhanced Magnetic Composite Gel for Highly Efficient Dye Adsorption and Catalysis,” ACS Sustainable Chemistry & Engineering, Vol. 3, No. 7, 2015, pp. 1677-1685.
  •  
  • 6. Mani, S.K., and Bhandari, R., “Microwave-assisted Synthesis of Self-assembled Network of Graphene Oxide-Polyethylenimine-Polyvinyl Alcohol Hydrogel Beads for Removal of Cationic and Anionic Dyes from Wastewater,” Journal of Molecular Liquids, Vol. 345, 2022, pp. 117809.
  •  
  • 7. Han, M., Xu, B., Zhang, M., Yao, J., Li, Q., Chen, W., and Zhou, W., “Preparation of Biologically Reduced Graphene Oxide-based Aerogel and Its Application in Dye Adsorption,” Science of the Total Environment, Vol. 783, 2021, 147028.
  •  
  • 8. Choi, Y.H., Lee, S.S., Lee, D.M., Jeong, H.S., and Kim, S.H., “Composite Microgels Created by Complexation between Polyvinyl Alcohol and Graphene Oxide in Compressed Double‐Emulsion Drops,” Small, Vol. 16, No. 9, 2020, pp. 1903812.
  •  
  • 9. Chang, Z., Chen, Y., Tang, S., Yang, J., Chen, Y., Chen, S., Li, P., and Yang, Z., “Construction of Chitosan/polyacrylate/graphene Oxide Composite Physical Hydrogel by Semi-dissolution/acidification/sol-gel Transition Method and Its Simultaneous Cationic and Anionic Dye Adsorption Properties,” Carbohydrate polymers, Vol. 229, 2020, pp. 115431.
  •  
  • 10. Mittal, H., Al Alili, A., Morajkar, P.P., and Alhassan, S.M., “Graphene Oxide Crosslinked Hydrogel Nanocomposites of Xanthan Gum for the Adsorption of Crystal Violet Dye,” Journal of Molecular Liquids, Vol. 323, 2021, pp. 115034.
  •  
  • 11. Guo, H., Jiao, T., Zhang, Q., Guo, W., Peng, Q., and Yan, X. “Preparation of Graphene Oxide-based Hydrogels as Efficient Dye Adsorbents for Wastewater Treatment,” Nanoscale Research Letters, Vol. 10, No. 1, 2015, pp. 1-10.
  •  
  • 12. Wang, N., Chang, P.R., Zheng, P., and Ma, X., “Graphene–poly (vinyl alcohol) Composites: Fabrication, Adsorption and Electrochemical Properties,” Applied Surface Science, Vol. 314, 2014, pp. 815-821.
  •  
  • 13. Lee, J.J., “Characteristics of Isotherm, Kinetic and Thermodynamic Parameters for the Adsorption of Acid Red 66 by Activated Carbon,” Clean Technology, Vol. 26, No. 1, 2020, pp. 30-38.
  •  
  • 14. Cho, S., “Fabrication of Functional Microcapsules Using Microfluidic Approach and Their Application to Heavy Metal Ions Adsorption,” MS Thesis, Chonnam National University, KR, 2021.
  •  
  • 15. Cho, S., Kim, J.H., Yang, K.S., and Chang, M., “Facile Preparation of Amino-functionalized Polymeric Microcapsules as Efficient Adsorbent for Heavy Metal Ions Removal,” Chemical Engineering Journal, Vol. 425, 2021, pp. 130645.
  •  
  • 16. Sun, L., Wang, J., Yu, Y., Bian, F., Zou, M., and Zhao, Y., “Graphene Oxide Hydrogel Particles from Microfluidics for Oil Decontamination,” Journal of Colloid and Interface Science, Vol. 528, 2018, pp. 372-378.
  •  

This Article

Correspondence to

  • Changhun Yun, Mincheol Chang

  • * Department of Polymer Engineering, Graduate School, Chonnam National University, Gwangju 61186, Korea
    ** School of Polymer Science and Engineering, Chonnam National University, Gwangju 61186, Korea

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